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Levels of ambient particulate matter have become the focus of increased attention over recent years as a result of studies suggesting an association between exposure and adverse health effects. Whilst research is continuing in many areas to identify a biological mechanism whereby this association can be explained, as yet there are only hypotheses. Causal relationships between observed health effects (i.e. increased hospital admissions, mortality, respiratory or heart problems) and any specific characteristic of the ambient aerosol have yet to be confirmed. Ambient aerosol has a complex chemistry and a wide range of physical properties, most of which undergo constant modification or transformation within the atmosphere. The particles in this aerosol may have originated either from natural or anthropogenic sources and may be either primary emissions (i.e. directly emitted to the atmosphere as particles) or secondary particles - formed by reaction of gas phase components.

Six European vehicles fitted with carbon canisters have been tested under severe conditions to establish if evaporative losses of volatile organic compounds occur under European driving conditions - so-called “running losses”. The programme entailed the development of a point source measurement technique which has a number of advantages over other methods currently in use. Following the development and validation of the measurement technique, the six vehicles were tested at 28C over a range of driving cycles on a gasoline with a Reid vapour pressure of 90 kPa. None of the vehicles exhibited classical running losses, i.e. losses during higher-speed driving. This was due to the effectiveness of canister purging in these conditions. However, significant volatile organic compound (VOC) losses were observed for several vehicles during idle after a period of driving had heated the fuel. Substantial car-to-car variation was observed in the losses obtained.