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Technical Paper

High-Resolution Transmission Electron Microscopy of Soot Directly Sampled at Different Axial Locations in Diesel Spray Flame

2011-09-11
2011-24-0068
For better understanding of soot formation and oxidation processes in a diesel spray flame, morphology, microstructure and size of soot particles directly sampled at different locations in the spray flame (40mm to 90mm from injector nozzle tip) were investigated using a high-resolution transmission electron microscope (HRTEM). The diesel spray flame was achieved in a constant volume combustion chamber under diesel-like conditions (2.5MPa and 940K). The concentration, diameter of primary particles and the radius of gyration of soot aggregates increased in the upstream region (40 to 50mm), exhibited a peak around the mid-stream region (60 to 70mm), and then decreased in the downstream region (80 to 90mm) from the injector nozzle tip, which corresponds to formation, peak concentration and oxidation of soot particles in the spray flame, respectively.
Journal Article

Direct Sampling, TEM Analysis and Optical Measurement of Soot Particles at Different Axial Locations in a Transient Spray Flame

2011-08-30
2011-01-2051
In order for better understanding of soot formation and oxidation processes in diesel spray flame, the morphology, microstructure and sizes of soot particles directly sampled in a transient spray flame were analyzed via high-resolution transmission electron microscopy (HRTEM). The soot distribution in the spray flame was simultaneously observed by high-speed shadowgraphy. The transient spray combustion was achieved in a constant volume combustion chamber under a high pressure and high temperature condition (940 K, 2.5 MPa). The soot samples were taken at different axial locations in the spray flame, 40 - 90 mm from the injector nozzle, using an intrusive soot sampler. Pressure histories, heat release rates and laser shadowgraphs of spray combustion were compared between the cases with and without the soot sampler in order to check the intrusion effect of soot sampler on combustion.
Technical Paper

Transmission Electron Microscopy of Soot Particles sampled directly from a Biodiesel Spray Flame

2011-08-30
2011-01-2046
For better understanding of soot formation and oxidation processes in a biodiesel spray flame, the morphology, microstructure and sizes of soot particles directly sampled in a spray flame fuelled with soy-methyl ester were investigated using transmission electron microscopy (TEM). The soot samples were taken at different axial locations in the spray flame, 40, 50 and 70 mm from injector nozzle, which correspond to soot formation, peak, and oxidation zones, respectively. The biodiesel spray flame was generated in a constant-volume combustion chamber under a diesel-like high pressure and temperature condition (6.7 MPa, 1000K). Density, diameter of primary particles and radius of gyration of soot aggregates reached a peak at 50 mm from the injector nozzle and was lower or smaller in the formation or oxidation zones of the spray.
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