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The development of new generations of internal combustion engines requires appropriate measurement techniques for all relevant limited exhaust gas species and particulates. However, because of stricter future emission limits, there is a severe lack especially with respect to soot particles. Conventional methods, like gravimetric sampling, have substantial deficiencies in sensitivity and temporal resolution, which is strongly required for transient tests. Furthermore, artifacts arise from other exhaust components, like sulfuric acid, water vapor and volatile hydrocarbons. In contrast to the state-of-the-art techniques, laser induced incandescence (LII) has been proved to be a favorable technique, which overcomes these deficiencies and offers additional information, which allows new insight into combustion phenomena. Besides soot mass concentration, also the soot primary particle size is accessible by this technique.

Improved understanding of the active combustion chain “injection - vaporisation - mixture formation - ignition - combustion - exhaust gas emissions” is important for the further development of IC engines with respect to fuel consumption and pollutant emissions. By means of multidimensional optical, mostly laser-based measurement techniques, a modern passenger car common rail system, applied to an optically accessible engine, was investigated. The utilisation of a new optical detection system allowed a simultaneous detection of the liquid phase by Mie scattering, the flame propagation from flame luminosity and the soot formation by laser-induced incandescence inside the combustion bowl of the engine. By such simultaneous measurements, direct dependencies of single combustion phenomena on fuel injection parameters can be resolved, and in particular soot formation and oxidation can be correlated to the actual combustion situation.

In previous work, time-resolved laser-induced incandescence (TIRE-LII) has been introduced as a favorable and easy-to-use technique for accurate online measurements of soot within the exhaust gas of production engines without modifications and first experimental results have been presented. The method relies on the detection of the thermal radiation of the particles after heating with a high power laser pulse. Additionally to soot concentration measurements, a simultaneous determination of soot primary particle sizes and, derived from these, also of the particle number concentrations is possible. Basic features of the technique are the high temporal resolution, which also makes transient tests feasible, and its high sensitivity and selectivity. These aspects suggest its application as a standard method for exhaust measurements with enhanced performance, which also leads to considerable new insight into internal combustion phenomena.

Ultrafine particles within Diesel exhaust gases have gained increased attention within the last few years, as especially the particle size is expected to be the key property for possible toxicity and carcinogenicity from Diesel engine emission. Various exhaust aftertreatment systems like oxidizing catalysts or soot filters have been applied for a significant reduction of soot mass concentration, but their influence on particle sizes and number concentration also has to be considered. This enhances the need for new measurement techniques which allow to measure relevant morphological parameters of soot particles. Laser-induced incandescence (LII) is presented as a favorable optical technique for soot measurements.