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Contaminated air and process gases, whether in a crewed spacecraft cabin atmosphere, the working volume of a microgravity science or ground-based laboratory experiment facility, or the exhaust from an automobile, are pervasive problems that ultimately effect human health, performance, and well-being. The need for highly-effective, economical decontamination processes spans a wide range of terrestrial and space flight applications. Adsorption processes are used widely for process gas decontamination. Most industrial packed bed adsorption processes use activated carbon because it is cheap and highly effective. Once saturated, however, the adsorbent is a concentrated source of contaminants. Industrial applications either dump or regenerate the activated carbon. Regeneration may be accomplished in-situ or at an off-site location. In either case, concentrated contaminated waste streams must be handled appropriately to minimize environmental impact.

An integrated sorber-based Trace Contaminant Control System (TCCS) and Carbon Dioxide Removal Assembly (CDRA) prototype was designed, fabricated and tested. It corresponds to a 1-person load. Performance over several adsorption/regeneration cycles was examined. Vacuum regenerations at effective time/ temperature conditions, and estimated power requirements were experimentally verified for the combined CO2/trace contaminant removal prototype. The current paper details the design and performance of this prototype during initial testing at CO2 and trace contaminant concentrations in the existing CDRA, downstream of the drier. Additional long-term performance characterization is planned at NASA. Potential system design options permitting associated weight, volume savings and logistic benefits, especially as relevant for long-duration space flight, are reviewed.

The development of energy efficient, lightweight sorption systems for removal of environmental contaminants in space flight applications is an area of continuing interest to NASA. The current CO2 removal system on the International Space Station employs two pellet bed canisters of 5A molecular sieve that alternate between regeneration and sorption. A separate disposable charcoal bed removes trace contaminants. An alternative technology has been demonstrated using a sorption bed consisting of metal meshes coated with a sorbent, trademarked and patented [1] as Microlith® by Precision Combustion, Inc. (PCI); these meshes have the potential for direct electrical heating for this application. This allows the bed to be regenerable via resistive heating and offers the potential for shorter regeneration times, reduced power requirement, and net energy savings vs. conventional systems. The capability of removing both CO2 and trace contaminants within the same bed has also been demonstrated.

The International Space Station (ISS) Trace Contaminant Control Subassembly (TCCS) design is based upon proven, highly reliable technology. However, because its core unit operations rely upon expendable activated charcoal and an indirectly heated high temperature catalyst, annual logistics mass, crew time, and power consumption requirements are significant. To address this situation, a unique catalytic reactor design has been developed which is suitable for retrofit into the TCCS’s high temperature catalytic oxidizer (HTCO) assembly. The unique design, which employs a metallic, ultra-short channel length monolith (USCM) catalyst substrate, was tested in a flight-like TCCS HTCO assembly to investigate its performance characteristics. Test results indicate that retrofitting the TCCS with a USCM-based catalytic reactor is feasible and that it may provide significant reductions in logistics mass, crew time, and power consumption.

The Trace Contaminant Control Subassembly (TCCS) to be used onboard the International Space Station (ISS) uses expendable adsorption beds and a conventional high temperature catalytic oxidizer to control trace chemical contaminants in the cabin air. Although effective, the current design has a high life cycle operating cost associated with maintaining the expendable beds and heating the catalytic oxidizer. In order to improve the TCCS's process economics, a retrofit to its primary design is being studied which utilizes an advanced technology lightweight, long-life Microlith™ catalytic converter (MCC). Development and testing of MCC prototypes for application to the TCCS have been conducted on a bench scale. Results from these studies are presented that show the converter's destruction performance for representative trace chemical contaminants found in a spacecraft cabin atmosphere.

This paper reports test results of a compact, high pollutant conversion efficiency, catalytic muffler developed for utility engines (<19kW/25hp). Tests were conducted in-house, and at an independent laboratory under EPA supervision and funding, using a four-stroke engine generator set. The specific HC, CO and NOx emissions were reduced by 98%, 97%, and 19%, respectively. This level of reduction is thought to be sufficient for reducing such emissions from utility engines to the level of future standards such as 1999 CARB. A total of 200 hours of performance and limited durability testing were accumulated on the catalytic muffler. The prototype demonstrated successful operation by entraining fresh air and mixing with exhaust gas, converting pollutants, maintaining acceptable skin and exhaust gas temperatures, and muffling noise.