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Planar laser-induced fluorescence (PLIF) has been successfully used for the investigation of the mixture formation process in hydrogen engines. Detailed information has been obtained about the process development (qualitative measurements) and on the fuel/air-ratio (quantitative measurements) in the combustion chamber. These results can be used for further optimization of the mixture formation and the combustion process concerning emissions and fuel consumption. The measurement technique used here is not limited to hydrogen and can also be applied to other fuel gases like natural gas. The main topic of this paper is the experimental verification of the PLIF data by simultaneous Raman scattering measurements. By Raman scattering the fuel/air-ratio can directly be determined from the direct concentration measurements of the different gas species.

The optimization of the vaporization and mixture formation process is of great importance for the development of modern gasoline direct injection (GDI) engines, because it influences the subsequent processes of the ignition, combustion and pollutant formation significantly. In consequence, the subject of this work was the development of a measurement technique based on the laser induced exciplex fluorescence (LIF), which allows the two dimensional visualization and quantification of the in-cylinder air/fuel ratio. A tracer concept consisting of benzene and triethylamine dissolved in a non-fluorescent base fuel has been used. The calibration of the equivalence ratio proportional LIF-signal was performed directly inside the engine, at a well known mixture composition, immediately before the direct injection measurements were started.

The influence of exhaust gas recirculation (EGR) on the formation of nitric oxide (NO) was studied experimentally in a transparent gasoline direct injection engine by quantitative laser-induced fluorescence imaging. Spectral properties of the excited transition within the NO A2∑+-X2∏(0,2) band are well known from previous studies. The excitation scheme allows quantitative NO concentration measurements without detailed knowledge of the gas phase temperature. Good agreement was found with exhaust gas NOx chemi-luminescence (CLD) measurements. The experiments were carried out in an optically accessible gasoline engine featuring a direct injection cylinder head (BMW) and a Bosch injection system, based on a serial inline six-cylinder engine with an enlarged crankcase. The measurements were performed in the pentroof section of the combustion chamber.

The formation of nitric oxide in a transparent direct injection gasoline engine was studied experimentally using two different schemes of laser-induced fluorescence (LIF) with KrF excimer (248 nm) excitation. With detection of the fluorescence shifted towards the red, strong interference from fluorescence of partially burned fuel was found. With blue-shifted fluorescence, interference was minimized allowing selective detection of NO. Possibilities of quantifying NO fluorescence intensities in inhomogeneous combustion are discussed.