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With the aim of elucidating the mechanism generating knock, an examination was made of the preflame reaction behavior of end gas in the combustion chamber in the transition from normal combustion to abnormal combustion characterized by the occurrence of knocking. Simultaneous measurements were made in the same cycle of the light absorption and emission behavior of the OH (characteristic spectrum of 306.4 nm), CH (431.5 nm) and C2 (516.5 nm) radicals in the end-gas region using spectroscopic methods. The absorbance behavior of a blue flame prior to autoignition is believed to be an important factor in the mechanism causing knock.

With the aim of elucidating the mechanism causing abnormal combustion, a study was made of light emission and absorption characteristics at wavelengths corresponding to the spectra of the OH (characteristic spectrum of 306.4 nm), CH (431.5 nm), C2 (516.5 nm) radicals. Spectral properties were measured in the end-gas region of the cylinder for various types of fuel having different octane numbers. During combustion in an actual engine, the behavior of the CH and C2 radicals prior to the occurrence of abnormal combustion characterized by knock is indicative of behavior in the negative temperature coefficient (NTC) region. The experimental results revealed that the behavior of the OH, CH, C2 radicals differs between normal and abnormal combustion.