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Effects of measurement method, coolant temperature and fuel composition on soot emissions were examined by engine experiments. By reducing the pressure fluctuation in the sampling line, the measured soot emissions with better stability and reproducibility could be obtained. With lower coolant temperatures, larger soot emissions were yielded at much advanced fuel injection timings. Compared to gasoline, soot emissions with a blend fuel of normal heptane, isooctane and toluene were significantly decreased, suggesting the amounts of aromatic components (toluene or others) should be increased to obtain a representative fuel for the predictive model of particulate matter in SIDI engines.

Suppression or reduction of soot emissions is an important goal in the development of automotive engines for environmental and human health purposes. A better understanding at the molecular level of the formation process of soot particles resulting from collision and aggregation of smaller particles made of Polycyclic Aromatic Hydrocarbon (PAH) is needed. In addition to experiments, computational methods are efficient and valuable tools for this purpose. As a first step in our detailed computational chemistry study, we applied Ultra-Accelerated Molecular Dynamics (UAQCMD) and Canonical Monte-Carlo (CMC) methods to investigate the nucleation process. The UA-QCMD can calculate chemical reaction dynamics 107 times faster than conventional first principle molecular dynamics methods, while CMC can calculate equilibrium properties at various temperatures, pressures, and chemical compositions.

We developed a novel ignition method called laser breakdown-assisted long-distance discharge ignition (LBALDI) that combines laser breakdown with a discharge to realize lean combustion. The creation of laser breakdown plasma between electrodes for discharge enables discharges over longer distances than those of conventional sparkplug as inferred from laser-triggered lightning or laser-triggered gas switches. This method should help realize volumetric ignition through the creation of a long-distance discharge. Experiments on the fundamental discharge and ignition of methane/air mixtures were conducted. The optimum incident time of the laser prior to the application of a high voltage was found to reduce the sparkover voltage and markedly reduce the voltage required by LBALDI under pressurized air conditions. In the ignition experiment, LBALDI showed the fastest heat release rate at the lean flammable limit.

A novel diagnostic technique named a “Tracer-Producing LIF technique” which enables 2-dimensional measurement of an internal EGR within an engine cylinder, has been developed. The main feature of this technique is the utilization of a fuel additive that does not itself emit an LIF signal by irradiation of UV-light but whose combustion products radiate strong LIF emissions by UV-light irradiation. Internal EGR behaviors can be measured by observing LIF images that are excited by a UV-laser sheet. Firstly, principles of this technique were confirmed and fuel additives were selected. Then, the “Tracer-Producing LIF technique” was applied to an optically accessible single-cylinder gasoline engine in which the entire pent-roof area can be observed from the side of the engine. The internal EGR behaviors were measured through the entire engine cycle, from intake to exhaust.

Over the last few decades, in-cylinder visualization using optically accessible engines has been an important tool in the detailed analysis of the in-cylinder phenomena of internal combustion engines. However, most current optically accessible engines are recognized as being limited in terms of their speed and load, because of the fragility of certain components such as the elongated pistons and transparent windows. To overcome these speed and load limits, we developed a new generation of optically accessible engines which extends the operating range up to speeds of 6000 rpm for the SI engine version, and up to in-cylinder pressures of 20 MPa for the CI engine version. The main reason for the speed limitation is the vibration caused by the inertia force arising from the heavy elongated piston, which increases with the square of the engine speed.

A computational and experimental study has been carried out to assess the high load efficiency and emissions potential of a combustion system designed to operate on low octane gasoline (or naphtha). The “naphtha engine” concept utilizes spark ignition at low load, HCCI at intermediate load, and compression ignition at high load; this paper focuses on high load (compression ignition) operation. Experiments were carried out in a single cylinder diesel engine with compression ratio of 16 and a common rail injector/fuel delivery system. Three fuels were examined: a light naphtha (RON∼59, CN∼34), heavy naphtha (RON∼66, CN∼31), and heavy naphtha additized with cetane improver (CN∼40). With single fuel injection near top dead center (TDC) (diesel-like combustion), excessive combustion noise is generated as the load increases. This noise limits the maximum power, in agreement with the CFD predictions. The noise-limited maximum power increases somewhat with the use of single pilot injection.

Natural gas homogeneous charge compression ignition (HCCI) engines require high compression ratios and intake air heating because of the high auto-ignition temperature of natural gas. In the first study, the natural gas fueled HCCI combustion with internal exhaust gas recirculation (EGR) was achieved without an intake air heater. The effects of the combustion chamber configuration, turbocharging, and external EGR were investigated for expanding the operating range. As a result, it was cleared that the combination of internal / external EGR and turbocharging is effective for expanding the HCCI operational range toward high loads. Meanwhile, the HCCI combustion characteristics at high engine speeds were unstable because of an insufficient reaction time for auto-ignition. Although the engine operation with a richer air-fuel ratio was effective for improving the combustion stability, the combustion noise (CN) was at an unacceptable level.

Two-line excitation LIF (Laser-Induced Fluorescence) technique for 2-dimensional temperature measurements in an engine cylinder before ignition is presented. From the fundamental examinations, the combination of toluene tracer with a pair of excitation lines of 248nm and 266nm has been selected because of the high LIF intensity ratio and closer excitation wavelengths. In-cylinder thermometry is conducted using a visualized single cylinder spark ignition engine both in PFI (port-fuel-injection) and DI (direct-injection) operation. The accuracy of this technique is determined through the homogeneous PFI experiment. Temperature and fuel distribution in unburned mixture are measured simultaneously in DI operation. It exists a strong correlation between equivalence ratio and temperature inside the mixture. Temperature in the fuel rich region is lower than in the fuel lean region.

The effects of fuel octane have been assessed on the efficiency and emissions of a high compression ratio (ε=13) spark ignition direct injection (SIDI) engine. Under low load stratified operation (1200 rpm, ∼20% load), a low octane fuel (RON=84, comprised of toluene, iso-octane, and n-heptane) yielded higher brake thermal efficiency and significantly lower hydrocarbon emissions than a base gasoline (RON=91). The indicator diagram for the low octane fuel showed evidence for two stage heat release, suggesting the presence of spark induced compression ignition (SICI). These results suggest that higher efficiency under low load stratified conditions can be obtained with lower octane fuels that undergo SICI combustion. The effect of fuel octane under high load was assessed at WOT with a high RON model fuel (RON=103, comprised of toluene, iso-octane, and n-heptane).

Recently, the smokeless rich diesel combustion had been demonstrated [1]. This can realize smokeless and NOx-less combustion by using a large amount of cooled EGR under a near stoichiometric and even in a rich operating condition. We focus on the effects of reducing diesel combustion temperature on soot reduction.

A multi-component fuel vaporization model is developed for numerical analysis of specific fuel component behaviors in port-fuel-injection(PFI) gasoline engines. In order to specify the differences of in-cylinder fuel distribution among its components, three-dimensional calculations of intake flow, spray and vapor motion of each component are performed with respect to engine wall temperature and the distillation characteristics of the fuel. Simultaneous measurements of in-cylinder behaviors of different volatility components in the fuel are also carried out using a laser-induced fluorescence (LIF) technique to validate the calculation results. In both measurements and calculations, the same fuels are used, which are composed of seven or eight components to simulate the distillation characteristics of two kinds of gasoline. The in-cylinder vapor amount of high and low volatility components is compared between the calculations and the experiments.

The effect of the chemical reactivity of diesel fuel on PM formation was investigated using a flow reactor and a shock tube. Reaction products from the flow-reactor pyrolysis of the three diesel fuels used for the engine tests in Part 1(1) (“Base”, “Improved” and Swedish “Class-1”) were analyzed by gas chromatography. At 850C, Swedish “Class-1” fuel was found to produce the most PM precursors such as benzene and toluene among the three fuels, even though it contains very low amounts of aromatics. The chemical analyses described in Part 1 revealed that “Class-1” contains a large amount of branched and cyclic structures in the saturated hydrocarbon portion of the fuel. These results suggest that the presence of such branched and ring structures can increase exhaust PM emissions.

NO laser-induced fluorescence (LIF) imaging and quantitative fuel distribution measurements in aport-fuel-injected 4-valve stratified-charge single-cylinder SI engine have been conducted using a tunable KrF excimer laser. The correlations between NO formation region and fuel distribution have been investigated for the horizontal stratification realized by fuel (iso-octane) injection in only one intake port. The NO LIF intensity is proportional to the exhaust NOx emissions. The strong NO LIF intensity region in expansion stroke corresponds to the location of the region with equivalence ratio (ϕ) between 0.8 and 1.1 in the stratified fuel distributions at spark timing. The exhaust NOx concentration is proportional to the area of region with ϕ =0.8 - 1.1.

This paper describes a laser-induced fluorescence (LIF) method for quantitative 2-D fuel concentration measurements in an SI engine. The combination of fluorescence tracer and excitation wavelength to lower the temperature and pressure effects on LIF intensity were evaluated. Each kind of fluorescence tracer selected from ketones, aldehydes and aromatics has been excited at 248 nm or 266 nm in a heated and pressurized constant volume vessel. For the promising candidates, further evaluation has been performed using a fired visualization engine. The results show that the optimum combination which gives the lowest effects of temperature and pressure on LIF intensity is acetone with 266 nm excitation. 3-pentanone, which is commonly used fluorescence tracer has been shown to be not suitable for the quantitative measurements, especially in a fired engine.

A reduced chemical kinetic model has been developed using temperature history measured by Coherent Anti-Stokes Raman Spectroscopy (CARS) and sensitivity analysis. Predictions of knock occurrence by this model show that the chemical role of residual gas and the intake flow have little effect on the knock occurrence crank angle. Furthermore, the effectiveness of the combustion period and the unburned gas temperature before spark ignition on the torque at trace knock limit (TTKL) has been clarified Under certain conditions, it is shown that the increase in torque, caused by the combustion duration shortened by ∼25%, is negated by the temperature rise of ∼15K before spark ignition.