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Planar laser-induced fluorescence (PLIF) has been successfully used for the investigation of the mixture formation process in hydrogen engines. Detailed information has been obtained about the process development (qualitative measurements) and on the fuel/air-ratio (quantitative measurements) in the combustion chamber. These results can be used for further optimization of the mixture formation and the combustion process concerning emissions and fuel consumption. The measurement technique used here is not limited to hydrogen and can also be applied to other fuel gases like natural gas. The main topic of this paper is the experimental verification of the PLIF data by simultaneous Raman scattering measurements. By Raman scattering the fuel/air-ratio can directly be determined from the direct concentration measurements of the different gas species.

The optimization of the vaporization and mixture formation process is of great importance for the development of modern gasoline direct injection (GDI) engines, because it influences the subsequent processes of the ignition, combustion and pollutant formation significantly. In consequence, the subject of this work was the development of a measurement technique based on the laser induced exciplex fluorescence (LIF), which allows the two dimensional visualization and quantification of the in-cylinder air/fuel ratio. A tracer concept consisting of benzene and triethylamine dissolved in a non-fluorescent base fuel has been used. The calibration of the equivalence ratio proportional LIF-signal was performed directly inside the engine, at a well known mixture composition, immediately before the direct injection measurements were started.

Mie-Scattering and laser induced exciplex fluorescence (LIEF) were used to visualize the distribution of liquid fuel and fuel vapor inside an optical accessible one-cylinder research engine with gasoline direct injection (GDI). Using a tracer which was developed especially for the environments of gasoline combustion engines, LIEF enables an extensive separation between liquid and vapor phase and delivers a signal proportional to the equivalence ratio. Simultaneous images of LIEF and Mie scattering proof the high quality of the phase separation using this tracer concept. The mixture formation process will be shown exemplary at one operation point with homogeneous load and another with stratified load. First results of determining the air/fuel ratio by means of linear Raman spectroscopy will be presented and compared with the two-dimensional qualitative distribution of the fuel vapor (LIEF).

The vapor phase of an evaporating spray from a heavy-duty Diesel common-rail injection system has been investigated with an optical diagnostic technique based on linear Raman scattering, which has been extended to the application in fuel sprays. One-dimensional spatially resolved Raman measurements of the air/fuel-ratio have been performed in the spray region with high local and temporal resolution in an injection chamber at an air pressure of 4.5 MPa and at a temperature of 450°C. The influence of different parameters, such as rail pressure, nozzle geometry and injection duration on the temporal evolution of the local air/fuel-ratio in the vapor phase has been studied quantitatively, and results from a selected spatial location are compared. Furthermore, the effect of physical/chemical fuel properties on the evaporation dynamics has been investigated by performing measurements with two different fuels.