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Carbon fiber reinforced plastic (CFRP) composites have gained particular interests due to their high specific modulus, high strength, lightweight and resistance to environment. In the automotive industry, numerous studies have been ongoing to replace the metal components with CFRP for the purpose of weight saving. One of the significant benefits of CFRP laminates is the ability of tailoring fiber orientation and ply thickness to meet the acceptable level of structural performance with little waste of material capability. This study focused on the concurrent optimization of ply orientation and thickness for CFRP laminated engine hood, which was based on the gradient-based discrete material and thickness optimization (DMTO) method. Two manufactural constraints, namely contiguity and intermediate void constraints, were taken into account in the optimization problem to reduce the potential risk of cracking matrix of CFRP.