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Dimethyl ether (DME) appears to be an attractive alternative to common fossil fuels in compression ignition engines due to its smokeless combustion and fast mixture formation. However, in order to fully understand the complex combustion process of DME, there is still a remaining need to develop a comprehensive chemical kinetic mechanism that includes both soot and NOx chemistry. In this study, a detailed DME mechanism with 305 species is developed from the basic DME mechanism of Curran et al. (2000) with addition of soot and NOx chemistry from Howard's mechanism et al. (1999), and GRI 3.0 mechanism, respectively. Soot chemistry in Howard mechanism consisting hydrogen abstraction acetylene addition (HACA) and growth of small polycyclic aromatic hydrocarbons (PAH), assesses over a wide range of temperature and is able to predict good to fair the formation of PAH up to coronene.

An operational scheme with fuel-lean and exhaust gas dilution in spark-ignited engines increases thermal efficiency and decreases NOx emission, while these operations inherently induce combustion instability and thus large cycle-to-cycle variation in engine. In order to stabilize combustion variations, the development of an advanced ignition system is becoming critical. To quantify the impact of spark-ignition discharge, ignitability tests were conducted in an optically accessible combustion vessel to characterize the flame kernel development of lean methane-air mixture with CO₂ simulating exhaust diluent. A shrouded fan was used to generate turbulence in the vicinity of J-gap spark plug and a Variable Output Ignition System (VOIS) capable of producing a varied set of spark discharge patterns was developed and used as an ignition source. The main feature of the VOIS is to vary the secondary current during glow discharge including naturally decaying and truncated with multiple strikes.

Water spray characterization of a multi-hole injector under pressures and temperatures representative of engine-relevant conditions was investigated for naturally aspirated and boosted engine conditions. Experiments were conducted in an optically accessible pressure vessel using a high-speed Schlieren imaging to visualize the transient water spray. The experimental conditions included a range of injection pressures of 34, 68, and 102 bar and ambient temperatures of 30 - 200°C, which includes flash-boiling and non-flash-boiling conditions. Transient spray tip penetration and spray angle were characterized via image processing of raw Schlieren images using Matlab code. The CONVERGE CFD software was used to simulate the water spray obtained experimentally in the vessel. CFD parameters were tuned and validated against the experimental results of spray profile and spray tip penetration measured in the combustion vessel (CV).

Particular matter (PM) has been greatly concerned over the recent decades due to the constantly increasing restriction on its effect on environmental aspect. Oxygenated fuel such as dimethyl ether (DME) has been known to have beneficial impact on diesel engine emissions in terms of zero soot formation. In current study, under several ambient conditions including surrounding gas temperature and oxygen percentages, soot and emission formation of DME spray is investigated to provide a comparison with other diesel surrogate (n-heptane) and JP-8 surrogate fuels. One important work is to develop a number of chemical kinetic mechanisms with soot chemistry including the growth of polycyclic aromatic hydrocarbon (PAH) and nitro oxides (NOx) formation. Using the developing detailed mechanisms, several numerical approaches were introduced to provide an integrated picture of emission formations.