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The interaction of fuel sprays with in-cylinder air flow is crucially important for the mixture preparation and subsequent combustion processes in gasoline direct injection (GDI) engines. In the present work, the experimentally validated computational fluid dynamics (CFD) simulations are performed to study the dynamics and physical insight of hollow-cone sprays interacting with a uniform crossflow. The basis of the model is the standard Reynolds-averaged Navier-Stokes (RANS) approach coupled to the Lagrangian treatment for statistical groups (parcels) representing the physical droplet population. The most physically suitable hybrid breakup models depicting the liquid sheet atomization and droplet breakup processes based on the linear instability analysis and Taylor analogy theory (LISA-TAB) are used. Detailed comparisons are made between the experiments and computations in terms of spray structure, local droplet diameter and velocity distributions.