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Selective catalytic reduction (SCR) of oxides of nitrogen (NOx) with gaseous ammonia is the leading technology used to meet on- and off-highway NOx emission standards across the world. In typical SCR systems, a low-pressure injector introduces a solution of urea and water (UWS) into hot exhaust gases leading to atomization and subsequent spray processes that finally lead to production of gaseous ammonia. Through their synergetic effect, the UWS injector and mixing enhancement devices (such as static mixers or baffles) help deliver a uniform mixture of ammonia and NOx to the SCR catalyst with minimal urea-derived solid deposits. To develop an efficient and robust aftertreatment system, it is essential to have experimental and simulation capabilities to assess the behavior of sprays under flow conditions representative of engine exhaust.

The combustion propagation mechanism of homogeneous charge compression ignition combustion was investigated using planar laser Rayleigh scattering thermometry, and was compared to that of spark-ignition combustion. Ethylene and dimethyl ether were chosen as the fuels for SI and HCCI experiments and have nearly constant Rayleigh scattering cross-sections through the combustion process. Beam steering at the entrance window limited the load range for HCCI conditions and confined the quantitative interpretation of the results to local regions over which an effective beam steering correction could be applied. The SI conditions showed a clear bimodal temperature behavior with a well-defined interface between reactants and products. The HCCI results showed large regions that were partially combusted, i.e., at a temperature above the reactants but below the adiabatic flame temperature. Dual-imaging experiments confirm that the burned region was progressing towards the fully burned state.

Reactivity controlled compression ignition combustion was investigated for three fuel combinations: isooctane-diesel, PRF90-diesel, and E85-diesel. Experiments were conducted at 1200 rpm, 160 kPa absolute intake pressure, and fixed total fuel energy using ‘optimal’ operating condition for each fuel combination that were chosen based on combustion performance from SOI timing and premixed energy fraction sweeps. The heat release duration was found to scale with the difference in reactivity between the premixed and direction injected fuel; a small difference gives rise to short heat release duration, similar to that of HCCI combustion. Conversely, as the difference increases, the heat release period lengthens. The high-speed optical data confirmed that the combustion occurred in a staged manner from the high-reactivity zones, which were located at the periphery of the chamber, to low-reactivity zones in the field of view.