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Solid particle emissions from a modern gasoline hybrid electrical vehicle (HEV) and a conventional gasoline vehicle were studied under diverse transient drive cycles on a chassis dynamometer. It is found that solid particle emissions from the conventional gasoline vehicle which has a 3.8-liter engine are sensitive to vehicle temperatures. Over 90% of solid particles are emitted during the first 250 seconds of transient cycles. Spikes for solid particle emissions from the HEV during a transient cycle are mainly caused by engine starts, hard accelerations after engine starts, and the engine running harder at high vehicle speeds. The engine and vehicle temperature status on the HEV doesn't show a strong correlation to the solid particle emission.

On-board Particulate Matter (PM) mass calibration (OB-PMMC) is an approach to calibrate a real-time PM sensor with the gravimetric PM mass being collected on a conventional filter. The real-time PM sensor is integrated in a PM sample system and takes sample upstream of the sample filter. The PM mass collected on the filter is determined either by weighing the filter or by using analytical approaches. A unique calibration coefficient for each sample filter is generated for converting the PM real-time signal to the real-time PM mass emission. This calibration approach can be used to modify Constant Volume Samplers (CVS) and laboratory Partial Flow Sample Systems (PFSS), etc., into real-time PM mass measurement instruments for engine or vehicle exhaust PM measurement. The same technique may also be used to measure real-time PM concentration in the atmosphere under some circumstance.

Two Euro 4 light-duty diesel vehicles were retrofitted with Diesel Particulate Filters (DPF). One was retrofitted with a low efficiency flow-through DPF. And, the other was retrofitted with a high efficiency wall-flow DPF. PM emissions from both vehicles were evaluated under the new European drive cycle (NEDC) on a chassis dynamometer. Several instruments were used to measure particulate matter (PM) emissions simultaneously from different aspects for two retrofitted vehicles. The PM mass emission from the vehicle retrofitted with the low efficiency DPF is close to 5.0 mg/km Euro 5 mass emission standard. However, the solid particle number emission is about 30 times higher than the Euro 5 solid particle number emission standard. Mass and number emissions from the vehicle retrofitted with the high efficiency DPF are well below Euro 5 emission standards.

An on-board diesel particulate measurement (OBS-TRPM) instrument is developed to measure on-road exhaust PM emission at Horiba. It is used to characterize particulate matter (PM) emission from a gasoline vehicle, the 1999 Ford Windstar with California Ultra Low Emission (ULEV) certification. PM emissions from three test cycles, EPA FTP 72, SFTP-US06, and new European drive cycle (NEDC), are evaluated. It is found that the PM emission from the SFTP-US06 with the cold start is roughly two times higher than PM emissions from the cold FTP 72 and the cold NEDC. This may be due to aggressive drive patterns for the US06 while the vehicle is still cold. The aggressive drive pattern for the US06 makes the gasoline vehicle emit a much higher fraction of elemental carbon (EC), and lower fraction of organic carbon (OC). Fractions of the EC from the vehicle are 9.1% for the FTP 72, 6.3% for the NEDC, and 56.6% for the US06.

The on-board transient response diesel particulate measurement (OBS-TRPM) instrument measures on-road vehicle particulate emissions. It is a continuation of the Horiba on-board PM sampler (OBS-PM) [5]. The OBS-TRPM measures total diesel particulate emission by collecting diesel particulate matter (PM) on a pre-weighed 47 mm filter while the partial flow sample system (OBS-PM) runs under a proportional control strategy. A real-time diffusion charge sensor (DCS) takes sample upstream of the filter, and measures diesel PM in term of particle length (mm/cm3). By integrating the DCS real-time signal during the filter sampling, the cumulative fraction of diesel PM emission is obtained. Finally, diesel PM mass emission during a specific region, for example a Not-to-Exceed (NTE) zone, is calculated from the fraction of the real-time PM signal. Thus, the OBS-TRPM provides a solution to measure PM emission in NTE zones which are defined by the US EPA.

Monodisperse and polydisperse Sodium Chloride (NaCl) particles were used to calibrate the solid particle penetration for the Volatile Particle Remover (VPR) in a Horiba prototype Solid Particle Counting System (SPCS). Prior to the calibration, dilution ratios on the SPCS are verified carefully with a flame ionization analyzer (FIA). Size distributions for polydisperse aerosols upstream and downstream of the Volatile Particle Remover (VPR) were measured with a Scanning Mobility Particle Sizer (SMPS). It is found that overall penetrations for polydisperse aerosols are larger than 95%. Geometric standard deviations from the raw and the diluted by the VPR are within ±1.5% difference. Thus, shapes of size distributions aren't changed after dilution. Geometric mean diameters shift a little, on average ±5% after dilution. Therefore, the VPR doesn't change the aerosol characteristics after the aerosol is diluted and heated up to 320 °C.

Horiba on-board diesel exhaust particulate sampler (OBS-PM) is a filter based partial flow particulate sampling system used for On-board diesel particulate matter (PM) measurement. It takes sample from either raw or diluted exhaust. It can run at constant dilution ratios or at variable dilution ratios with proportional control on the sample flow. The diluted exhaust moves through a pre-weighed 47 mm particulate filter and PM is collected on the filter. By weighing the loaded sample filter, PM emission from the engine or the vehicle can be determined. The performance of the OBS-PM meets most of requirements for a real-time partial flow sample system (PFSS) recommended by ISO 16183 [2]. The physical size and the power consumption of the instrument are minimized. It is powered with four 12 volts batteries, and can be installed on a vehicle for real-world PM emission evaluation.

A Solid Particle Counting System (SPCS) has been developed according to the ECE draft regulation proposed by the particle measurement program (PMP). In the previous report the basic performance of the SPCS has been mentioned in detail [1, 2, 3, 4, 5 and 6]. It has been reported that the SPCS demonstrates very stable dilution of sample with air and the error of real time dilution factor is less than 6% up to the total dilution factor of 1000. Penetration of solid particles through the SPCS is over 95% and volatile particles removal efficiency is over 99%. In this study the SPCS has been used to investigate the soot emission behavior from different vehicles with different after-treatment technologies. Direct injection (DI) diesel vehicles without diesel particulate filter (DPF), and with different DPFs (catalyzed and non-catalyzed) have been tested. Direct injection gasoline (DIG) vehicle with oxidation and NOx reduction catalysts have also been tested.

The prototype solid particle counting system (SPCS) has been used to study solid particle emission from gasoline and diesel vehicles. As recommended by the PMP draft proposal, exhaust is diluted by a Constant Volume Sampler (CVS). The SPCS takes the sample from the CVS tunnel. Transient test cycles such as EPA FTP 75, EPA HWFET (EPA Highway Fuel Economy Cycle), and NEDC (New European Driving Cycle) were tested. The repeatability of the instrument was evaluated on the diesel vehicle for three continuous days. The instrument exhibits good repeatability. The differences for the EPA ftp 75, the EPA HWFET, and the NEDC in three continuous tests are ± 3.5%. The instrument is very sensitive as well and detects the driving differences. A large number of solid particles are found during the hard acceleration from both the gasoline and the diesel vehicles. Solid particle emissions decrease quickly at deceleration and when vehicles approach constant speed.

A prototype solid particle counting system (SPCS) has been developed in Horiba. It measures the engine exhaust solid particle number emissions in real-time. The instrument is designed to follow the recommendation in the PMP proposal for solid particle number emissions measurement on Light-duty diesel vehicles. Two wide range continuous diluters, which were developed during this project, have been used as cold and hot diluters, respectively. The accuracy of the dilution ratio is normally ± 4% for the designed range. The instrument has low particle losses, and exhibits over 95% penetration for solid particles. The new instrument has functions such as, normal measurement, dilution ratio control, daily calibration for condensation particle counter (CPC), etc. These functions have been automated to make the instrument's operation simple.

A one-stage dilution tunnel has been developed to sample and dilute diesel exhaust. The tunnel has the capability of simulating many aspects of the atmospheric dilution process. The dilution rate and overall dilution ratio, temperature, relative humidity, and residence time in the tunnel, as well as residence time and temperature in the transfer line between the tunnel and exhaust sampling point may be varied. In this work we studied the influence of the exhaust transfer line, tunnel residence time, and dilution air temperature on the exhaust particle size distribution. The influences of fuel sulfur content on the size distribution and on the sensitivity of the size distribution to dilution and sampling conditions were also examined. We do not suggest an optimum dilution scheme, but do identify critical variables.

A single-stage dilution system has been designed to simulate the process of engine exhaust dilution in the atmosphere. An exhaust sample stream is introduced into a partial flow tunnel where it is diluted at a controlled rate. Temperature, relative humidity, dilution ratio and rate, and residence time are all adjustable. The system includes a turbulence generator to adjust the intensity of turbulence in the tunnel and a wake disk to control the initial mixing rate. Numerical methods were used to simulate flow fields, velocity fields, and mixing profiles for gases and particles. Mixing profiles for a gaseous tracer and particles of different sizes were also determined experimentally and compared with the model predictions. Critical parameters that influence mixing profiles and dilution rates predicted by modeling were demonstrated experimentally. Predicted and measured normalized mixing profiles were found to be in good agreement.